A visible-light-responsive metal-organic framework MIL-53(Fe) was synthesized.
LED lamps emitting white light were utilized as excitation light source.
The introduction of PS effectively suppressed the recombination of charge carriers.
The formed SO4− and OH radicals accelerated the photocatalytic degradation of AO7.
MIL-53(Fe) showed good reusability and high stability at near-neutral pH.