Carbide slag pellets were prepared via a novel extrusion–spheronization.
Two new pore-forming materials were used to enhance CO2 sorption of the pellets.
Addition of microcrystalline cellulose improves the CO2 sorption of the pellets.
Pellets doped with pre-washed rice husk are superior to those with raw rice husk.
The mechanical strength of the pellets could be enhanced via addition of cement.