A Silver–Organic Frameworks Based on Flexible-Aromatic Dicarboxylate and Bipyridinyl Skeletons Coligand: Crystal Structure and Luminescence Property
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- 作者：Ruo-Fei Bai ; Xun Feng ; Yi-Ling Sun…
- 关键词：d10 metal ; Flexible nitrogen ; heterocyclic acid ; Hydrogen bonds ; Luminescence ; Sensors
- 刊名：Journal of Inorganic and Organometallic Polymers and Materials
- 出版年：2016
- 出版时间：May 2016
- 年：2016
- 卷：26
- 期：3
- 页码：512-518
- 全文大小：2,210 KB
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Xun Feng (1)
Yi-Ling Sun (1) (2)
Hong Chen (1)
Guo-Zhan Qin (1)
Xin-Fang Liu (1)
1. College of Chemistry and Chemical Engineering, Luoyang Normal University, Luoyang, 471022, China
2. College of Chemistry and Molecular Engineering, Zhengzhou University, Zhengzhou, 450001, China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Inorganic Chemistry
Organic Chemistry
Polymer Sciences - 出版者：Springer New York
- ISSN：1574-1451
文摘
Reaction between silver salt and conjugational N-hetrocyclic carboxylic acid with the presence of bipyridyl skeletons auxiliary ligand afforded a d10 metal polymer namely [(ddpp)Ag(bipy) (1)] (ddpp = 2, 5-di(2′,4′-dicarboxylphenyl)pyridine, bipy = 4,4′-bipyridine). It was characterized by elements analysis, infrared spectroscopy, single crystal X-ray diffraction and thermogravimetry studying. For the polymer 1, silver centers are three coordinated geometry with an ON2 donor set provided by ddpp and bipy. The polymer 1 is built from 1-D alternative/zig-zag chain, as the secondary building unit, and further stacks via hydrogen bonds which formed between two isophthalic moieties of ddpp ligands and weak interactions to generate a two-dimensional, 2D supramolecular layer. Moreover, the polymer 1 displays thermal stability in solid state and the luminescence behaviour is also investigated in a dimethyl sulphoxide solution at ambient temperature, and it also can be applied in design of sensors to detect of trace aluminum, zinc and calcium ion.