Effect of Different Carbon Substrates on the Removal of Hexahydro-1,3,5-Trinitro-1,3,5-Triazine (RDX) and Octahydro-1,3,5,7-Tetranitro-1,3,5,7-Tetrazocine (HMX) by Anaerobic Mesophilic Granular Sludge

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• 作者：Chunjiang An ; Yarong Shi ; Yanling He ; Guohe Huang…
• 关键词：Hexahydro ; 1 ; 3 ; 5 ; trinitro ; 1 ; 3 ; 5 ; triazine (RDX) ; Octahydro ; 1 ; 3 ; 5 ; 7 ; tetranitro ; 1 ; 3 ; 5 ; 7 ; tetrazocine (HMX) ; Degradation ; Mesophilic anaerobic granules ; Carbon substrates
• 刊名：Water, Air, and Soil Pollution
• 出版年：2014
• 出版时间：November 2014
• 年：2014
• 卷：225
• 期：11
• 全文大小：584 KB
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• 作者单位：Chunjiang An (1) (2)
  Yarong Shi (1)
  Yanling He (2)
  Guohe Huang (1)
  Jidong Liang (2)
  Zongkuan Liu (3)
  
  1. Institute for Energy, Environment and Sustainable Communities, University of Regina, Regina, Saskatchewan, S4S 0A2, Canada
  2. School of Energy and Power Engineering, Xi’an Jiaotong University, Xi’an, 710049, People’s Republic of China
  3. School of Human Settlement and Civil Engineering, Xi’an Jiaotong University, Xi’an, 710049, People’s Republic of China
  
• ISSN：1573-2932

文摘

The influence of carbon substrate supplement on the degradation of hexahydro-1,3,5-trinitro-1,3,5-triazine (RDX) and octahydro-1,3,5,7-tetranitro-1,3,5,7-tetrazocine (HMX) by anaerobic mesophilic granular sludge was investigated. Batch experiments were carried to evaluate the biodegradation performance in the presence of acetate, ethanol, glucose and soluble starch. The results of specific methanogenic activity tests showed that RDX and HMX at concentration of 139 and 20?μmol?L?, respectively, had no major inhibitory effect on the bioactivity of anaerobic granular sludge. Glucose and acetate could better facilitate the degradation of RDX and HMX when compared with ethanol and soluble starch. The concentration of carbon substrate was considered critical for enhancing the transformation of RDX and HMX. As carbon substrate concentration increased up to 50?mmol chemical oxygen demand (COD) L?, there was a major stimulatory effect of the amended carbon substrates, while a slight inhibitory effect was also found at some concentrations. These results indicate that adding suitable carbon substrates may be an important strategy for stimulating the anaerobic biotransformation of high-energetic ammunition compounds in bioreactors.