Rare Earth Pincer Complexes: Synthesis, Reaction Chemistry, and Catalysis

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• 关键词：Catalysis ; Lanthanides ; Pincer ligands ; Rare earth metals ; Reactivity
• 刊名：Topics in Organometallic Chemistry
• 出版年：2016
• 出版时间：2016
• 年：2016
• 卷：54
• 期：1
• 页码：93-177
• 全文大小：5,765 KB
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• 作者单位：Mikko M. Hänninen (15)
  Matthew T. Zamora (15)
  Paul G. Hayes (15)
  
  15. Department of Chemistry and Biochemistry, University of Lethbridge, 4401 University Dr W, Lethbridge, AB, Canada, T1K 3M4
  
• 丛书名：The Privileged Pincer-Metal Platform: Coordination Chemistry & Applications
• ISBN：978-3-319-22927-0
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Organometallic Chemistry
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1616-8534

文摘

The research field surrounding rare earth pincer complexes has reached a stage where a comprehensive review about the reactivity and catalytic behavior of these species is justified. In this contribution, we begin with a brief introduction on common strategies for the preparation of rare earth pincer complexes, continuing with a section devoted to the versatile reactivity observed for this class of compound. Thereafter, several types of compounds are discussed, including extremely reactive hydrides, cationic species, and intriguing scandium imido complexes. Finally, the last portion of this chapter sums up the hitherto reported catalytic studies, including discussions on ring-opening polymerization of cyclic esters, polymerization of olefins and hydroamination reactions, as well as several examples of more infrequently encountered catalytic processes.