Cellulose-based nanostructures for photoresponsive surfaces

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• 作者：Susete N. Fernandes ; Luis E. Aguirre ; Rita V. Pontes ; João P. Canejo…
• 关键词：Cellulose derivatives ; Photoresponsive structures ; Wettability ; Tunable interfacial templates ; Nanofilaments
• 刊名：Cellulose
• 出版年：2016
• 出版时间：February 2016
• 年：2016
• 卷：23
• 期：1
• 页码：465-476
• 全文大小：1,398 KB
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• 作者单位：Susete N. Fernandes (1)
  Luis E. Aguirre (1)
  Rita V. Pontes (1)
  João P. Canejo (1)
  Pedro Brogueira (2)
  Eugene M. Terentjev (3)
  Maria H. Godinho (1)
  
  1. I3N/CENIMAT, Department of Materials Science, Faculty of Sciences and Technology, Universidade NOVA de Lisboa, Campus da Caparica, 2829-516, Caparica, Portugal
  2. Physics Department and ICEMS, Instituto Superior Técnico, ULisboa, Av. Rovisco Pais, 1, 1049-001, Lisbon, Portugal
  3. Cavendish Laboratory, University of Cambridge, JJ Thomson Avenue, Cambridge, CB3 0HE, UK
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Bioorganic Chemistry
  Physical Chemistry
  Organic Chemistry
  Polymer Sciences
  
• 出版者：Springer Netherlands
• ISSN：1572-882X

文摘

Cellulose is the main constituent of plant cell walls and can be converted into a wide range of derivatives. The derivatives are produced by a chemical reaction of the primary and two secondary hydroxyl groups available in β-d-glucopyranose units, often in heterogeneous conditions, yielding, in many cases, <3 average degrees of substitution per glucose unit. Here we profit from the richness of these systems and different assembly conditions building up from similar nanomicelles, with a characteristic length of ca. 30 nm, different nanostructures: lamellas and filaments that show dissimilar responses to UV irradiation. The chosen cellulose derivative was a thermotropic liquid crystal synthesized by the reaction of 4-(4-methoxyazobenzene-4′-yloxy)butanoyl chloride and acetoxypropylcellulose. The nanostructures were obtained from this cellulose derivative by using spin-coating as well as Langmuir–Blodgett techniques. The nanostructures with a high surface-to-volume ratio, which can be freestanding or grown off a substrate, lead to organic tunable interfacial templates with distinct wettability properties. Keywords Cellulose derivatives Photoresponsive structures Wettability Tunable interfacial templates Nanofilaments