Effects of additives on dissolution of cellobiose in aqueous solvents
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- 作者：Zhijing Liu ; Chao Zhang ; Ruigang Liu ; Wushou Zhang ; Hongliang Kang ; Ning Che…
- 关键词：Cellulose ; Interactions ; Aqueous solution ; Additive ; Dissolution
- 刊名：Cellulose
- 出版年：2015
- 出版时间：June 2015
- 年：2015
- 卷：22
- 期：3
- 页码：1641-1652
- 全文大小：1,530 KB
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Roshind MU, Tahtinen P, Ni - 作者单位：Zhijing Liu (1) (4)
Chao Zhang (1) (4)
Ruigang Liu (1)
Wushou Zhang (2)
Hongliang Kang (1)
Ning Che (1) (4)
Pingping Li (1) (4)
Yong Huang (1) (3)
1. State Key Laboratory of Polymer Physics and Chemistry, Beijing National Laboratory of Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
4. University of Chinese Academy of Sciences, Beijing, 100049, China
2. CAS Key Laboratory of Colloid, Interface and Chemical Thermodynamics, Institute of Chemistry, Chinese Academy of Sciences, Beijing, 100190, China
3. National Research Center for Engineering Plastics, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing, 100190, China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Bioorganic Chemistry
Physical Chemistry
Organic Chemistry
Polymer Sciences - 出版者：Springer Netherlands
- ISSN：1572-882X
文摘
Cellobiose was used as a model compound for cellulose to study dissolution in aqueous systems with additives. The dissolution of cellobiose in alkali solutions is a typical exothermic enthalpy-driven process, confirming that lower temperature is beneficial for dissolution of cellulose in NaOH aqueous systems. OH?/sup> plays an important role in cellobiose dissolution by forming cellobiose–OH?/sup> hydrogen-bonded complexes. The ability to form hydrogen bonds between additives and cellobiose in aqueous solutions follows the order NaOH/urea/ZnO?>?NaOH/urea/NaAlO2?>?NaOH/urea?>?NaOH. Direct interactions between OH?/sup>, amino groups of urea, Na+ hydrates, and?cellobiose result in stable hydrogen-bonding complexes among cellobiose, OH?/sup>, Na+ hydrates, and urea. Addition of ZnO or NaAlO2 can promote the dissolution power of the solvent system for cellulose. This work clarifies the interactions and dissolution mechanisms of cellulose in aqueous solution systems with additives through hydrogen-bonding interactions.