Arsenic Adsorption and its Fractions on Aquifer Sediment: Effect of pH, Arsenic Species, and Iron/Manganese Minerals

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• 作者：Jie Ma ; Huaming Guo ; Mei Lei ; Xiaoyong Zhou ; Fulan Li…
• 关键词：Arsenic ; Adsorption ; Fraction ; Aquifer sediments ; pH ; Arsenic species ; Fe/Mn minerals
• 刊名：Water, Air, and Soil Pollution
• 出版年：2015
• 出版时间：August 2015
• 年：2015
• 卷：226
• 期：8
• 全文大小：2,661 KB
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• 作者单位：Jie Ma (1) (2) (3)
  Huaming Guo (1) (2)
  Mei Lei (3)
  Xiaoyong Zhou (3)
  Fulan Li (1) (2)
  Tian Yu (1) (2)
  Rongfei Wei (3)
  Hanzhi Zhang (3)
  Xi Zhang (3)
  Yang Wu (3)
  
  1. State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Beijing, 100083, People鈥檚 Republic of China
  2. School of Water Resources and Environment, China University of Geosciences, Beijing, 100083, People鈥檚 Republic of China
  3. Center for Environmental Remediation, Institute of Geographic Sciences and Natural Resources Research, Chinese Academy of Sciences, Beijing, 100101, People鈥檚 Republic of China
  
• 刊物类别：Earth and Environmental Science
• 刊物主题：Environment
  Environment
  Atmospheric Protection, Air Quality Control and Air Pollution
  Waste Water Technology, Water Pollution Control, Water Management and Aquatic Pollution
  Terrestrial Pollution
  Hydrogeology
  
• 出版者：Springer Netherlands
• ISSN：1573-2932

文摘

Effects of pH, As species, and Fe/Mn minerals on the fractions of adsorbed As in aquifer sediments were evaluated. Kinetic data showed that As adsorption was controlled by diffusion through the external film. Isothermal data of both As(III) and As(V) fitted the Langmuir isotherm well, revealing a monolayer adsorption process. Sequential extraction demonstrated that water-soluble As and non-specifically sorbed As were the major fractions of adsorbed As. Assessing the relationship between the Freundlich K F and the increases in the amounts of As fractions showed that the pH played a key role in weakly adsorbed As, especially water-soluble As. Although inorganic As species converted each other during the adsorption processes, more non-specifically sorbed As was adsorbed in As(V)-treated sediment than in As(III)-treated sediment, showing that the electrostatic selectivity controlled the non-specific adsorption. Additionally, specifically sorbed As and As associated with the amorphous phases were predominated by Fe/Mn minerals, especially Fe(III) (hydr)oxides. These results suggested that pH, As species, and Fe/Mn minerals would regulate the As fractions in aquifer sediments, and therefore control As cycling in aquifer systems.