Influence of phosphorous addition on Bi3Mo2Fe1 oxide catalysts for the oxidative dehydrogenation of 1-butene
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- 作者：Jung-Hyun Park ; Chae-Ho Shin
- 关键词：Butadiene ; Oxidative Dehydrogenation ; Bi3Mo2Fe1P x Oxide Catalyst ; 1 ; C4H8 ; temperature ; programmed Desorption ; Temperature ; programmed Re ; oxidation
- 刊名：Korean Journal of Chemical Engineering
- 出版年：2016
- 出版时间：March 2016
- 年：2016
- 卷：33
- 期：3
- 页码：823-830
- 全文大小：459 KB
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Chae-Ho Shin (2)
1. Division of Physical Science and Engineering, KAUST Catalysis Center (KCC), King Abdullah University of Science and Technology (KAUST), 4700 KAUST, Thuwal, 23955-6900, Saudi Arabia
2. Department of Chemical Engineering, Chungbuk National University, Chungbuk, 28644, Korea - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Industrial Chemistry and Chemical Engineering
Catalysis
Materials Science
Biotechnology - 出版者：Springer New York
- ISSN：1975-7220
文摘
Bi3Mo2Fe1P x oxide catalysts were prepared by a co-precipitation method and the influence of phosphorous content on the catalytic performance in the oxidative dehydrogenation of 1-butene was investigated. The addition of phosphorous up to 0.4mole ratio to Bi3Mo2Fe1 oxide catalyst led to an increase in the catalytic performance; however, a higher phosphorous content (above P=0.4) led to a decrease of conversion. Of the tested catalysts, Bi3Mo2Fe1P0.4 oxide catalyst exhibited the highest catalytic performance. Characterization results showed that the catalytic performance was related to the quantity of a π-allylic intermediate, facile desorption behavior of adsorbed intermediates and ability for re-oxidation of catalysts.