Preparation, characterization and ion-exchange behavior of polyantimonic acid-polyacrylonitrile (PAA–PAN) composite beads for strontium(II)
详细信息 查看全文
- 作者：Fuyin Ma ; Wanlong Shi ; Hu Meng ; Zheng Li…
- 关键词：Polyantimonic acid ; polyacrylonitrile ; Modification ; Strontium(II) ; Adsorption isotherms ; Irradiation stability
- 刊名：Journal of Radioanalytical and Nuclear Chemistry
- 出版年：2016
- 出版时间：April 2016
- 年：2016
- 卷：308
- 期：1
- 页码：155-163
- 全文大小：1,211 KB
- 参考文献：1.IAEA (2002) Issues and trends in radioactive waste management. Proceeding Series, STI/PUB/1175, IAEA, Vienna
2.Kige PJ (2013) Latest radioactive leak at Fukushima: how is it different? http://news.nationalgeographic.com/news/energy/2013/08/130821
3.Zhang Anyunq, Kuraoka Etsushu, Kumagai Mikio (2007) Development of the chromatographic partitioning of cesium and strontium utilizing two macroporous silica-based calix[4]arene-crown and amide impregnated polymeric composites: PREC partitioning process. J Chromatogr A 1157:85–95CrossRef
4.Zhang Anyun, Wei Yuezhou, Hoshi Harutaka, Kumagai Mikio (2005) Chromatographic Separation of Strontium (II) from a Nitric Acid Solution Containing some Typically Simulated Elements by a Novel Silica-Based TODGA Impregnated Polymeric Composite in the MAREC Process. Solvent Extr Ion Exc 23:231–247CrossRef
5.Yuezhou Wei (2011) Progress and Discussion on Chemical Separation Technologies for Nuclear Fuel Reprocessing Developed Abrosd. Progr Chem 23(7):1272–1288
6.Hitoshi MIMURA, Kenichi AKIBA (1994) Separation of heat-generating nuclides from high-level liquid wastes through zeolite columns. J Nucl Sci Technol 31:463–469CrossRef
7.Fourie HO, Ghijsels JP (1969) Radiostrontium in biological material: precipitation and extraction procedure eliminating the use of fuming nitric acid. Health Phys 17(5):685–689CrossRef
8.Tian Guoxin (2005) Extraction of strontium from HLLW using N,N,N′,N′-tetraisobutyl 3-oxa-glutaramide. Solvent Extr Ion Exch 23:519–528CrossRef
9.Riddle CL, Baker JD, Law JD, McGrath CA (2005) Fission product extraction (FPEX): development of a novel solvent for the simultaneous separation of strontium and cesium from acidic solutions. Solvent Extr Ion Exch 23:449–461CrossRef
10.Romanovskiy VN, Smirnov IV (2001) The universal solvent extraction (UNEX) process I development of the UNEX process solvent for the separation of cesium, strontium, and the actinides from acidic radioactive waste. Solvent Extr Ion Exch 19(1):1–21CrossRef
11.Philip Horwitz E, Chiarizia R, Dietz ML (1992) A novel strontium-selective extraction chromatographic resin. Solvent Extr Ion Exch 10(2):313–336CrossRef
12.Inan Suleyman, Nostar Emine (2013) Structure and ion exchange behavior of zirconium antimonates for strontium. Sep Sci Technol 48:1364–1369CrossRef
13.Mushtaq A (2004) Inorganic ion-exchangers: their role in chromatographic radionuclide generators for the decade 1993–2002. J Radioanal Nucl Chem 262(3):797–810CrossRef
14.Sylvester Paul, Beherns Elizabeth A (1999) An assessment of inorganic ion-exchange materials for the removal of strontium from simulated Hanford tank wastes. Sep Sci Technol 34(10):1981–1992CrossRef
15.Zouad S, Loos-Neskovic C, Fedoroff M (1987) Fixation of strontium on polyantimonic acid. J Radioanal Nucl Chem 111:337–349CrossRef
16.Weng H, Li T (1982) Separation of 90Sr from 1AW wastes with polyantimonic acids. Chin J Nucl Sci Eng Sep 29(5):238–244
17.Sebesta F (1997) Composite sorbents of inorganic ion-exchangers and polyacrylonitrile binding matrix. J Radioanal Nucl Chem 220:77–88CrossRef
18.Suleyman S, Altas Y (2011) Preparation of zirconium–manganese oxide/polyacrylonitrile (Zr–Mn oxide/PAN) composite spheres and the investigation of Sr (II) sorption by experimental design. Chem Eng J 168:1263–1271CrossRef
19.Park Y, Lee Y-C, Shin WS, Choi S-J (2010) Removal of cobalt, strontium and cesium from radioactive laundry wastewater by ammonium molybdophosphate–polyacrylonitrile (AMP–PAN). Chem Eng J 162:685–695CrossRef
20.Nilchi A, Saberi R, Moradi M, Azizpour H, Zarghami R (2010) Evaluation of AMP–PAN composite for adsorption of Cs+ ions from aqueous solution using batch and fixed bed operations. J Radioanal Nucl Chem 292:609–617CrossRef
21.Moon J-K, Kim K-W, Jung C-H, Shul Y-G, Lee E-H (2000) Preparation of organic-inorganic composite adsorbent beads for removal of radionuclides and heavy metal ions. J Radioanal Nucl Chem 246:299–307CrossRef
22.Deng Q, Li M, Cheng Z (2008) Research on polyantimonic acid synthesis and adsorption for strontium. Nucl Powder Eng 29(5):142–145
23.Dwivedi C, Kumar A, Singh KK, Juby AK, Kumar M, Wattal PK, Bajaj PN (2013) Copper hexacyanoferrate-polymer composite beads for cesium ion removal: synthesis, characterization, sorption, and kinetic studies. J Appl Polym. doi:10.1002/APP.38707
24.Colomban P, Doremieux-Morin C (1989) Equilibrium between protonic species and conductivity mechanism in antimonic acid, H2Sb4O11·nH2O. J Mol Struct 213:83–96CrossRef
25.Sureshkumar MK, Das D, Mallia MB, Gupta PC (2010) Adsorption of uranium from aqueous solution using chitosan-tripolyphosphate (CTPP) beads. J Hazard Mater 184:65–72CrossRef
26.Das D, Das N, Mathew L (2010) Kinetics equilibrium and thermodynamic studies on biosorption of Ag(I) from aqueous solution by macrofungus Pleurotus platypus. J Hazard Mater 184:765–774CrossRef
27.Sivaiah MV, Venkatesan KA, Krishna RM, Sasidharb P, Murthy GS (2005) Ion exchange properties of strontium on in situ precipitated polyantimonic acid in amberlite XAD-7. Sep Purif Technol 44:1–9CrossRef - 作者单位：Fuyin Ma (1) (2) (3) (4)
Wanlong Shi (1) (2) (3) (4)
Hu Meng (1) (2) (3) (4)
Zheng Li (1) (3) (4)
Wei Zhou (1) (3) (4)
Lan Zhang (1) (3) (4)
1. Shanghai Institute of Applied Physics Chinese Academy of Science, Shanghai, 201800, China
2. University of Chinese Academy of Sciences, Beijing, 100049, China
3. Key Laboratory of Nuclear Radiation and Nuclear Energy Technology, Chinese Academy of Science, Shanghai, 201800, China
4. Center for Excellence TMSR Energy System, Chinese Academy of Science, Shanghai, 201800, China - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Nuclear Chemistry
Physical Chemistry
Nuclear Physics, Heavy Ions and Hadrons
Diagnostic Radiology
Inorganic Chemistry - 出版者：Akad茅miai Kiad贸, co-published with Springer Science+Business Media B.V., Formerly Kluwer Academic
- ISSN：1588-2780
文摘
An organic–inorganic composite ion exchanger of polyantimonic acid-polyacrylonitrile (PAA–PAN) was synthesized to remove strontium(II) from radioactive waste water. Ion exchange behavior of the composite toward strontium(II) were investigated and the results indicated that the composite presents excellent performance in 0.1 mol L−1 nitric acid. The maximum uptake capacity of strontium(II) can reach up to 49 mg g−1 on composite. Adsorption thermodynamic parameters showed that the ion exchange was endothermic and spontaneous reaction and equilibrium adsorption data fit well with the Langmuir adsorption isotherms. In addition, PAA–PAN beads were found to have chemical and adsorption stability under irradiation and acidic media.