Matryoshka-caged gold nanorods: Synthesis, plasmonic properties, and catalytic activity

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• 作者：Wei Xiong ; Debabrata Sikdar ; Lim Wei Yap ; Pengzhen Guo ; Malin Premaratne…
• 关键词：matryoshka ; caged gold nanorods ; galvanic replacement reaction ; 4 ; nitrophenol ; catalysis ; surface plasmon resonance
• 刊名：Nano Research
• 出版年：2016
• 出版时间：February 2016
• 年：2016
• 卷：9
• 期：2
• 页码：415-423
• 全文大小：2,933 KB
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• 作者单位：Wei Xiong (1) (2) (3)
  Debabrata Sikdar (4)
  Lim Wei Yap (1) (2)
  Pengzhen Guo (1) (2)
  Malin Premaratne (4)
  Xinyong Li (3)
  Wenlong Cheng (1) (2)
  
  1. Department of Chemical Engineering, Monash University, Clayton, VIC, 3800, Australia
  2. The Melbourne Centre for Nanofabrication, 151 Wellington Road, Clayton, VIC, 3168, Australia
  3. Key Laboratory of Industrial Ecology and Environmental Engineering and State Key Laboratory of Fine Chemicals, School of Environmental Sciences and Technology, Dalian University of Technology, Dalian, 116024, China
  4. Advanced Computing and Simulation Laboratory (AχL), Department of Electrical and Computer Systems Engineering, Monash University, Clayton, VIC, 3800, Australia
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chinese Library of Science
  Chemistry
  Nanotechnology
  
• 出版者：Tsinghua University Press, co-published with Springer-Verlag GmbH
• ISSN：1998-0000

文摘

Matryoshka-caged gold nanorods (mCGNRs) were successfully synthesized by alternating between a seed-mediated silver-coating method and galvanic replacement reactions (GRRs). As the number of matryoshka layers of the mCGNRs increased, the plasmon resonance peak broadened and was red-shifted, and the catalytic activity towards the reduction of 4-nitrophenol (4-NTP) increased. When mCGNRs with 6 layers were used as nanocatalysts in the reduction of 4-nitrophenol, the reaction rate coefficient was 5.2- and 3.7-times higher than that of the gold-nanorod- and caged-gold-nanorod-catalyzed reductions of 4-nitrophenol, respectively. In addition, the surface-plasmon-resonance-based absorption of light enhanced the catalytic performance of the mCGNRs. With the support of a polyurethane foam, the mCGNRs synthesized in this study can be applied as recyclable heterogeneous catalysts for the reduction of 4-nitrophenol.