Synthesis, characterization, and property testing of PGS/P(AMPS-co-AM) superabsorbent hydrogel initiated by glow-discharge electrolysis plasma

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• 作者：Jie Yu ; Haitao Zhang ; Yun Li ; Quanfang Lu ; Qizhao Wang…
• 关键词：Superabsorbent hydrogel ; Glow ; discharge electrolysis plasma (GDEP) ; Palygorskite (PGS) ; Graft copolymerization ; Swelling behavior ; Adsorption
• 刊名：Colloid & Polymer Science
• 出版年：2016
• 出版时间：February 2016
• 年：2016
• 卷：294
• 期：2
• 页码：257-270
• 全文大小：2,574 KB
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• 作者单位：Jie Yu (1)
  Haitao Zhang (1)
  Yun Li (1)
  Quanfang Lu (1) (2)
  Qizhao Wang (1)
  Wu Yang (1)
  
  1. Key Laboratory of Bioelectrochemistry and Environmental Analysis of Gansu Province, College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou, 730070, People’s Republic of China
  2. Editorial Department of the University Journal, Northwest Normal University, Lanzhou, 730070, People’s Republic of China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Polymer Sciences
  Physical Chemistry
  Soft Matter and Complex Fluids
  Characterization and Evaluation Materials
  Food Science
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1435-1536

文摘

A palygorskite/poly(2-acrylamido-2-methyl-1-propanesulfonic acid-co-acrylamide) (PGS/P(AMPS-co-AM)) superabsorbent hydrogel was prepared in aqueous solution using glow-discharge electrolysis plasma (GDEP) as an initiator and N,N′-methylene-bis-acrylamide as a cross-linker. A possible copolymerization mechanism initiated by GDEP was proposed. The structure, thermal stability, and morphology of PGS/P(AMPS-co-AM) were characterized by FT-IR, XRD, TG-DTG, and SEM. The swelling kinetics, pH-reversibility, and influence of various pH and salt solutions on the swelling were investigated. Adsorption kinetics and adsorption mechanism of hydrogel for dyes were studied in detail. The results indicated that the equilibrium swelling of hydrogel is 652.6 g g−1 in distilled water. The swelling of the hydrogel in salt solutions from highest to lowest is Na+ > Mg2+ > Fe3+. The hydrogel has pH-reversibility responsive to the pH and salts solutions. The adsorption process of dyes follows the pseudo-second-order kinetic model with multi-step diffusion process. In addition, PGS/P(AMPS-co-AM) hydrogel can be regenerated and reused. Keywords Superabsorbent hydrogel Glow-discharge electrolysis plasma (GDEP) Palygorskite (PGS) Graft copolymerization Swelling behavior Adsorption