Photocatalytic Decolorization of Dye Effluent Using Radiation Developed Polymeric Nanocomposites

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• 作者：Amr El-Hag Ali ; Amany I. Raafat…
• 关键词：Dye degradation ; Gamma radiation ; Nanocomposite ; Photocataysis ; ZnO
• 刊名：Journal of Inorganic and Organometallic Polymers and Materials
• 出版年：2016
• 出版时间：May 2016
• 年：2016
• 卷：26
• 期：3
• 页码：606-615
• 全文大小：1,474 KB
• 参考文献：1.M. Hassan, M.D. AlAhmadi, M. Mosaid, Arab. J. Chem. 8, 72 (2015)CrossRef
  2.S.-T. Lin, M. Thirumavalavan, T.-Y. Jiang, J.-F. Lee, Carbohydr. Polym. 105, 1 (2014)CrossRef
  3.I. Mallarda, L.W. Städe, S. Ruellan, P.A.L. Jacobsen, K.L. Larsen, S. Fourmentin, Colloids Surf. A Physicochem. Eng. Asp 482, 50 (2015)CrossRef
  4.A. Kumar, P. Choudhary, P. Verma, Chem. Pharm. Res. 4, 763 (2012)
  5.G.M. Nisola, E. Cho, A.B. Beltran, M. Han, Y. Kim, W. Chung, Chem. 80, 894 (2010)
  6.L. Fan, C. Luo, X. Li, F. Lu, H. Qiu, M. Sun, J. Hazard. Mater. 215–216, 272 (2012)CrossRef
  7.D. Pokhrel, T. Viraraghavan, J. Environ. Manage. 90, 1956 (2009)CrossRef
  8.Q.I. Rahman, M. Ahmad, S.K. Misra, M. Lohani, Mater. Lett. 91, 170 (2013)CrossRef
  9.X. Rong, F. Qiu, C. Zhang, L. Fu, Y. Wang, D. Yang, Powder Technol. 275, 322 (2015)CrossRef
  10.S.-Q. Li, H.P.-J. Zhou, W.-S. Zhang, H. Peng, J. Alloy Compd. 616, 227 (2014)CrossRef
  11.Y. Liu, S. Wei, W. Gao, J. Hazard. Mater. 287, 59 (2015)CrossRef
  12.B. Sultan, S. Nurettin, Polym. 52, 4834 (2011)CrossRef
  13.C. Sahoo, A.K. Gupta, J. Hazard. Mater. 215–216, 302 (2012)CrossRef
  14.Z. Ying, Z. Jian, Z. Xiulin, C. Zhenping, Radiat. Phys. Chem. 75, 485 (2006)CrossRef
  15.A. Bhattacharya, B.N. Misra, Prog. Polym. Sci. 29, 767 (2004)CrossRef
  16.Y.H.F. Al-qudah, G.A. Mahmoud, M.A. Abdel, Khalek. Res. Appl. Sci. 7, 135 (2014)
  17.S.G.A. Alla, H.M. Nizam El-Din, A.M. El-Naggar, Eur. Polym. J. 43, 2987 (2007)CrossRef
  18.M. Yadollahi, I. Gholamali, H. Namazi, M. Aghazadeh, Int. J. Biol. Macromol. 74, 136 (2015)CrossRef
  19.S. Jin, J. Gu, Y. Shi, K. Shao, X. Yu, G. Yue, Eur. Polym. J. 49, 1871 (2013)CrossRef
  20.B. Singh, V. Sharma, Int. J. Pharm. 389, 949 (2010)CrossRef
  21.S. Anitha, B. Balusamy, J. Thiruvadigal, T.S. Natarajan, Carbohydr. Polym. 87, 1065 (2012)CrossRef
  22.S. Shankar, X. Teng, G. Li, J. Rhim, Food Hydrocoll. 45, 264 (2015)CrossRef
  23.A. Nicolay, A. Lanzutti, M. Poelman, B. Ruelle, L. Fedrizzi, P. Dubois, M.-G. Olivier, Appl. Surf. Sci. 327, 379 (2015)CrossRef
  24.S. Bagheri, K.G. Chandrappa, S.B. Abd Hamid, Der. Pharma. Chem. 5, 265 (2013)
  25.X. Li, C. Hu, X. Wang, Y. Xi, Appl. Surf. Sci. 258, 4370 (2012)CrossRef
  26.N. Wetchakun, S. Chainet, S. Phanichphant, K. Wetchakun, Ceram. Int. 41, 5999 (2015)CrossRef
  27.N. Soltani, E. Saion, W.M.M. Yunus, M. Navasery, G. Bahmanrokh, M. Erfani, M.R. Zare, E. Gharibshahi, Sol. Energy 97, 147 (2013)CrossRef
  28.J.R. Reddy, S. Kurra, R. Guje, S. Palla, N.K. Veldurthi, G. Ravi, M. Vithaln, Ceram. Int. 41, 2869 (2015)CrossRef
  29.J. Zhao, X. Yang, Build. Environ. 38, 645 (2003)CrossRef
  30.D.P. Das, N. Biswal, S. Martha, K.M. Parida, J. Mol. Catal. A: Chem. 349, 36 (2011)CrossRef
  31.M. Chirita, I. Grozescu, Chem. Bull. 54, 1 (2009)
  32.A. Sadollahkhani, O. Nur, M. Willander, I. Kazeminezhad, V. Khranovskyy, M.O. Eriksson, R. Yakimova, P.-O. Holtz, Ceram. Inter. 41, 7174 (2015)CrossRef
  33.A. Bhattacharjee, M. Ahmaruzzaman, Mater. Lett. 145, 74 (2015)CrossRef
  34.L. Chen, C. Zhao, D.D. Dionysiou, K.E. O’Shea, J. Photochem. Photobiol. A Chem. 307–308, 115 (2015)CrossRef
  35.L.V. Barbosa, L. Marcal, E.J. Nassar, P.S. Calefia, M.A. Vicente, R. Trujillano, V. Rives, A. Gil, S.A. Korili, K.J. Ciuffi, E.H. de Faria, Catal. Today 246, 133 (2015)CrossRef
  36.S.F. Mohamed, G.A. Mahmoud, M.F. Abou, Taleb Monatsh. Chem. 144, 129 (2013)CrossRef
  
• 作者单位：Amr El-Hag Ali (1)
  Amany I. Raafat (1)
  Ghada A. Mahmoud (1)
  Nagwa A. Badway (2)
  M. A. El-Mottaleb (3)
  M. F. Elshahawy (1)
  
  1. National Center for Radiation Research and Technology, Atomic Energy Authority, P.O. Box 29, Nasr City, Cairo, Egypt
  2. Chemistry Department, Faculty of Science, Al-Azhar University, Nasr City, Cairo, Egypt
  3. Chemistry Department, Faculty of Science, Al-Azhar University, Assiut Branch, Asyût, Egypt
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Inorganic Chemistry
  Organic Chemistry
  Polymer Sciences
  
• 出版者：Springer New York
• ISSN：1574-1451

文摘

In this study [acrylic acid/p(N-vinyl-2-pyrrolidone)] (AAc/PVP) hydrogel was prepared using gamma irradiation technique. The prepared hydrogel was used as a template for in situ preparation of ZnO photocatalyst up to three deposition cycles. The structure, the thermal property, and the surface morphology of (AAc/PVP/ZnO) nanocomposite were characterized by X-ray diffraction (XRD), thermogravimetric analysis (TGA), transmission electron microscope (TEM) and scanning electron microscope (SEM) techniques. The photocatalytic activity of the obtained nanocomposite was tested for the degradation of methyl blue dye (MB) in the aqueous medium using UV-light. The effect of operational parameters on the degradation of MB such as UV irradiation time, pH, and initial dye concentration were examined. It was found that complete decolorization of MB dye was achieved after 45 min at pH 4. The degradation rate fitted the pseudo-first-order model and the rate of the photocatalytic reaction of the first preparation cycle of ZnO was higher than that of the third preparation cycle.