Behavior of PAH/mineral associations during thermodesorption: impact for the determination of mineral retention properties towards PAHs

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• 作者：Coralie Biache (1) (2)
  Catherine Lorgeoux (3) (4)
  Alain Saada (5)
  Pierre Faure (1) (2)
  
  1. Universit茅 de Lorraine ; LIEC ; UMR7360 ; 54506 ; Vand艙uvre-l猫s-Nancy ; France
  2. CNRS ; LIEC ; UMR7360 ; 54506 ; Vand艙uvre-l猫s-Nancy ; France
  3. Universit茅 de Lorraine ; GeoRessources ; UMR7359 ; 54506 ; Vand艙uvre-l猫s-Nancy ; France
  4. CNRS ; GeoRessources ; UMR7359 ; 54506 ; Vand艙uvre-l猫s-Nancy ; France
  5. BRGM ; 3 Avenue Claude Guillemin ; BP 36009 ; 45060 ; Orl茅ans Cedex 2 ; France
  
• 关键词：Evolved gas analysis ; Thermal desorption ; Bentonite ; Silica sand ; Polycyclic aromatic hydrocarbon ; Sorption
• 刊名：Analytical and Bioanalytical Chemistry
• 出版年：2015
• 出版时间：May 2015
• 年：2015
• 卷：407
• 期：12
• 页码：3509-3516
• 全文大小：1,787 KB
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• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Analytical Chemistry
  Food Science
  Inorganic Chemistry
  Physical Chemistry
  Monitoring, Environmental Analysis and Environmental Ecotoxicology
  
• 出版者：Springer Berlin / Heidelberg
• ISSN：1618-2650

文摘

Polycyclic aromatic hydrocarbons (PAHs) associated with two minerals (silica sand and bentonite) presenting opposite retention properties were analyzed with a thermodesorption (Td)-GC-MS coupling in order to validate this technique as a new and rapid way to evaluate the solid sorption properties. Two analysis modes were used, evolved gas analysis (EGA) and Td with cryo-trap. EGA allowed a real-time monitoring of the compounds desorbed during a temperature program and gave a first screening of the samples while Td gave more precise indications on compound abundances for selected temperature ranges. When associated with silica sand, PAHs were released at relatively low temperatures (PAHs were desorbed at much higher temperatures; they were also present in much lower abundance and were associated with mono-aromatic compounds. With bentonite, the PAH abundances decreased and the mono-aromatics increased with the increasing PAH molecular weight. These results indicated a clear PAH retention by the bentonite due to polymerization, followed by a thermal cracking at higher temperatures. The Td-GC-MS was proven to efficiently underline differences in retention properties of two minerals, and this study highlights the great potential of this technique to evaluate compound/matrix bond strength and interaction.