Scaled up low-temperature SOFCs with symmetrical electrode for applications
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- 作者：Huiqing Hu ; Qizhao Lin ; Xiangrong Liu ; Bin Zhu
- 关键词：Solid oxide fuel cells ; Samarium doped ceria ; Composite electrolyte ; Large size ; Engineering cell ; Symmetrical electrode
- 刊名：Journal of Solid State Electrochemistry
- 出版年：2015
- 出版时间：August 2015
- 年：2015
- 卷：19
- 期：8
- 页码：2361-2368
- 全文大小：937 KB
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Qizhao Lin (1)
Xiangrong Liu (2)
Bin Zhu (2)
1. Department of Thermal Science and Energy Engineering, University of Science and Technology of China, Jinzhai Road, Hefei, 230026, China
2. Department of Energy Technology, Royal Institute of Technology, Stockholm, 100 44, Sweden - 刊物类别：Chemistry and Materials Science
- 刊物主题：Chemistry
Physical Chemistry
Analytical Chemistry
Industrial Chemistry and Chemical Engineering
Characterization and Evaluation Materials
Condensed Matter
Electronic and Computer Engineering - 出版者：Springer Berlin / Heidelberg
- ISSN：1433-0768
文摘
In this study, a new type of the Mg0.4Zn0.6O/Ce0.8Sm0.2O2-δ (MZSDC) composite electrolyte was synthesized using a co-precipitation method. Large-sized engineering cells have been fabricated and tested to meet the demands of applications. X-ray diffraction scanning electron microscopy and X-ray photoelectron spectroscopy have been employed to characterize the microstructure and the morphology of the synthesized samples. MZSDC is a composite system. X-ray electron spectroscopy shows that Ce (3d) binding energy shifted from high to low and the ratio of Ce3+ decreased in comparison to pure CeO2, due to the doping effect. The doping and composite caused the material to have an excellent electrical property, 0.089?S?·?cm?, and device performance, with a maximum power of 16.4?W (648?mW?·?cm?) achieved at 600?°C for a larger-sized (6?cm?×-?cm?×-?mm) fuel cell. The open circuit voltage and power of the fuel cell only slightly degrades (less than 1?%) after continually tested for 100?h. This is the first report regarding the large size engineering cell performance for using this new composite electrolyte with both excellent performance and low cost.