Chirality assignment for metallic species via coherent phonon oscillations in arc-discharge single-walled carbon nanotubes

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• 作者：Seong-Il Shin ; Yong-Sik Lim ; Myung Jong Kim
• 关键词：Coherent phonon oscillations ; Arc ; discharge single ; walled carbon nanotubes ; Chirality assignment ; Spectral ; resolved spectroscopy
• 刊名：Journal of the Korean Physical Society
• 出版年：2015
• 出版时间：September 2015
• 年：2015
• 卷：67
• 期：5
• 页码：921-929
• 全文大小：960 KB
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• 作者单位：Seong-Il Shin (1)
  Yong-Sik Lim (1)
  Myung Jong Kim (2)
  
  1. Department of Nano Science and Mechanical Engineering, Konkuk University, Chungju, 380-701, Korea
  2. Soft Innovative Materials Research Center, Korea Institute of Science and Technology, Wanju, 565-905, Korea
  
• 刊物主题：Physics, general; Theoretical, Mathematical and Computational Physics; Particle and Nuclear Physics;
• 出版者：Springer Netherlands
• ISSN：1976-8524

文摘

We performed transient absorption measurements with sub-10-fs pulses to observe coherent phonon (CP) oscillations of species in a micelle-suspended arc-discharge single-walled carbon nanotube (SWNT) ensemble. We applied a spectral-resolved measurement scheme to investigate the photon-wavelength dependence of CP oscillations of the radial breathing mode (RBM) specific to each species, covering a broad photon wavelength range from 700 to 1000 nm (1.771 - 1.240 eV). With a linear prediction singular value decomposition (LPSVD) method as a robust alternative for resolving closely-overlapped vibration modes, we divided multiple RBM peaks into two components, the M ₁₁-excited metallic species and the S ₂₂-excited semiconducting species, respectively. We resolved the RBM peaks into 22 metallic and 29 semiconducting species. Resolved metallic tubes showed a wide distribution in diameters from 1.3 to 2.3 nm, forming a chirality distribution from (2n + m) = 33 family to 51 family. Keywords Coherent phonon oscillations Arc-discharge single-walled carbon nanotubes Chirality assignment Spectral-resolved spectroscopy