Study of viscoelastic properties of white carbon black reinforced synthetic polyisoprene

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• 作者：Guang-jun Cui ; Shi-wei Wang ; Peng-gang Yin…
• 关键词：Reinforcement ; White carbon black ; Synthetic polyisoprene ; Natural rubber ; Viscoelastic properties ; Payne effect
• 刊名：Chinese Journal of Polymer Science
• 出版年：2016
• 出版时间：April 2016
• 年：2016
• 卷：34
• 期：4
• 页码：457-465
• 全文大小：767 KB
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• 作者单位：Guang-jun Cui (1)
  Shi-wei Wang (1)
  Peng-gang Yin (1)
  Lin Guo 郭林 (1)
  
  1. Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology of Ministry of Education, School of Chemistry and Environment, Beihang University, Beijing, 100191, China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Condensed Matter Physics
  Industrial Chemistry and Chemical Engineering
  Polymer Sciences
  Characterization and Evaluation of Materials
  
• 出版者：Chinese Chemical Society and Institute of Chemistry, CAS, co-published with Springer
• ISSN：1439-6203

文摘

The viscoelastic properties of synthetic polyisoprenes (PI) reinforced by white carbon black (WCB) have been investigated and compared with WCB reinforced natural rubber (NR), including cure characteristics, physio-mechanical and dynamic mechanical properties. Compared with NR, PI loaded with the same amount of WCB (PI/WCB) exhibited shorter scorch time and optimal cure time, indicating that WCB fillers are comparatively easier to conjugate with PI. The tensile strength and elongation at break decreased with WCB filling in both PI and NR vulcanizates. The hardness of the rubber vulcanizates increased with the WCB filling in the rubber matrix. PI/WCB blends exhibited smaller hardness data, lower tensile strength, as well as lower elongation at break and tensile stress. Increasing the amount of WCB in rubber matrix induced the Payne effect. However, the Payne effect is much more obvious for the PI/WCB system, and PI/WCB also displayed higher storage modulus whereas lower loss modulus and loss tangent than NR/WCB, which could all be attributed to the poor dispersibilities of WCB in the PI matrix. Keywords Reinforcement White carbon black Synthetic polyisoprene Natural rubber Viscoelastic properties Payne effect