Soil contamination by polycyclic aromatic hydrocarbons at natural recreational areas in Delaware, USA

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• 作者：Shoujun Yuan (1)
  Kebin Li (2)
  Tianhu Chen (3)
  Xiaolong Bi (4)
  Qiquan Wang (5)
  
• 关键词：Polycyclic aromatic hydrocarbons (PAHs) ; Soil ; Contamination ; Natural recreational areas ; Delaware
• 刊名：Environmental Earth Sciences
• 出版年：2014
• 出版时间：July 2014
• 年：2014
• 卷：72
• 期：2
• 页码：387-398
• 全文大小：1,070 KB
• 参考文献：1. Abrahams PW (2002) Soils: their implications to human health. Sci Total Environ 291:1-1 CrossRef
  2. Agarwal T (2009) Concentration level, pattern and toxic potential of PAHs in traffic soil of Delhi, India. J Hazard Mater 171:894-00 CrossRef
  3. Agarwal T, Khillare PS, Shridhar V, Ray S (2009) Pattern, sources and toxic potential of PAHs in the agricultural soils of Delhi, India. J Hazard Mater 163:1033-039 CrossRef
  4. Banger K, Toor GS, Chirenje T, Ma L (2010) Polycyclic aromatic hydrocarbons in urban soils of different land uses in Miami, Florida. Soil Sediment Contam 19:231-43 CrossRef
  5. Blumer M (1961) Benzpyrenes in soil. Science 134:474-75 CrossRef
  6. Bryselbout C, Henner P, Carsignol J, Lichtfouse E (2000) Polycyclic aromatic hydrocarbons in highway plants and soils. Evidence for a local distillation effect. Analusis 28:290-93 CrossRef
  7. CCME (2007) Canadian soil quality guidelines for the protection of environmental and human health. Publication no. 1299, ISBN 1-896997-34-1. Canadian Council of Ministers of the Environment, Quebec
  8. Chung MK, Hu R, Cheung KC, Wong MH (2007) Pollutants in Hong Kong soils: polycyclic aromatic hydrocarbons. Chemosphere 67:464-73 CrossRef
  9. Delaware DAFS (2002) Forest health in delaware. Doc.# 65-1-4/06/10/02. Delaware Department of Agriculture Forest Service, Dover, DE. http://dda.delaware.gov/forestry/forest%20health%20report.pdf
  10. Delaware DNREC (2007) State resources area FAQs. Delaware: Delaware Department of Natural Resources and Environmental Control: Dover, DE. http://www.dnrec.delaware.gov/SiteCollectionDocuments/Open%20Spaces/SRA%20FAQS%20only%20%20REVISED%201.24.07.pdf
  11. Fontcuberta M, Arques JF, Martinez M, Suarez A, Villalbi JR, Centrich F, Serrahima E, Duran J, Casas C (2006) Polycyclic aromatic hydrocarbons in food samples collected in Barcelona, Spain. J Food Protect 69:2024-028
  12. Gigliotti CL, Dachs J, Nelson ED, Brunciak PA, Eisenreich SJ (2000) Polycyclic aromatic hydrocarbons in the New Jersey costal atmosphere. Environ Sci Technol 34:3547-554 CrossRef
  13. Glaser B, Dreyer A, Bock M, Fiedler S, Mehring M, Heitmann T (2005) Source apportionment of organic pollutants of a highway-traffic-influenced urban area in Bayreuth (Germany) using biomarker and stable carbon isotope signatures. Environ Sci Technol 39:3911-917 CrossRef
  14. Hwang HM, Green PG, Young TM (2006) Tidal salt marsh sediment in California, USA. Part 1: occurrence and sources of organic contaminants. Chemosphere 64:1383-392 CrossRef
  15. Itoh N, Aoyagi Y, Takatsu A, Yarita T (2009) Certified reference material for quantification of polycyclic aromatic hydrocarbons in sediment from National Metrology Institute of Japan. Anal Bioanal Chem 393:2039-049 CrossRef
  16. Jiang YF, Wang XT, Wang F, Jia Y, Wu MH, Sheng GY, Fu JM (2009) Levels, composition profiles and sources of polycyclic aromatic hydrocarbons in urban soil of Shanghai, China. Chemosphere 75:1112-118 CrossRef
  17. Kang Y, Cheung KC, Wong MH (2010) Polycyclic aromatic hydrocarbons (PAHs) in different indoor dust and their potential cytotoxicity based on two human cell lines. Environ Intern 36:542-47 CrossRef
  18. Keith LH, Telliard WA (1979) Priority pollutants I—a perspective view. Environ Sci Technol 13:416-23 CrossRef
  19. Kennaway E (1955) The identification of a carcinogenic compound in coal tar. British Med J 2:749-52 CrossRef
  20. Krauss M, Wilcke W (2003) Polychlorinated naphthalenes in urban soil: analysis, concentrations, and relation to other persistent organic pollutants. Environ Pollut 122:75-9 CrossRef
  21. Li Z, Sjodin A, Porter EN, Patterson DG Jr, Needham LI, Lee S, Russell AG, Mulholland JA (2009) Characterization of PM2.5-bound polycyclic aromatic hydrocarbons in Atlanta. Atmos Environ 43:1043-050 CrossRef
  22. Liang J, Ma GJ, Fang HL, Chen L, Christie P (2011) Polycyclic aromatic hydrocarbon concentrations in urban soils representing different land use categories in Shanghai. Environ Earth Sci 62:33-2 CrossRef
  23. Ma WL, Li YF, Sun DZ, Qi H (2009) Polycyclic aromatic hydrocarbons and polychlorinated biphenyls in topsoils of Harbin, China. Arch Environ Contam Toxicol 57:670-78 CrossRef
  24. Maliszewska-Kordybach B (1996) Polycyclic aromatic hydrocarbons in agricultural soils in Poland: preliminary proposals for criteria to evaluate the level of soil contamination. Appl Geochem 11:121-27 CrossRef
  25. Maliszewska-Kordybach B, Smreczak B, Klimkowicz-Pawlas A (2009) Effects of anthropopressure and soil properties on the accumulation of polycyclic aromatic hydrocarbons in the upper layer of soils in selected regions of Poland. Appl Geochem 24:918-926 CrossRef
  26. Naumova YY, Eisenreich SJ, Turpin BJ, Weisel CP, Morandi MT, Colome SD, Totten LA, Stock TH, Winter AM, Alimokhtari S, Kwon J, Shendell D, Jones J, Maberti S, Wall SJ (2002) Polycyclic aromatic hydrocarbons in the indoor and outdoor air in three cities in the U.S. Environ Sci Technol 36:2552-559 CrossRef
  27. Orecchio S (2010) Assessment of polycyclic aromatic hydrocarbons (PAHs) in soil of a natural reserve (Isola delle Femmine) (Italy) located in front of a plant for the production of cement. J Hazard Mater 173:358-68 CrossRef
  28. Quiroz R, Grimalt JO, Fernandez P, Camarero L, Catalan J, Stuchlik E, Thies H, Nickus U (2011) Polycyclic aromatic hydrocarbons in soils from European high mountain areas. Water Air Soil Pollut 215:655-66 CrossRef
  29. Smith DJT, Edelhauser EC, Harrison RM (1995) Polynuclear aromatic hydrocarbon concentrations in road dust and soil samples collected in the United Kingdom and Pakistan. Environ Technol 16:45-3 CrossRef
  30. Sun N, Lu CG, Gao X, Li CL, Chen LM (2007) Distribution and sources of polycyclic hydrocarbons (PAHs) in soil of East QingZang Plateau (in Chinese). Huanjing Kexue 28:664-68
  31. Takagi Y, Mineki S, Sera N, Nakahima D, Okatani AT, Kato Y, Kohzaki KI, Hisamatsu S, Goto S (2008) Measurement of concentrations of polycyclic aromatic hydrocarbons (PAHs) in sandboxes in 51 Japanese parks. Polycycl Aromat Comp 28:451-61 CrossRef
  32. US EPA (2012) Priority chemicals. National waste minimization program, US Environmental Protection Agency, Washington DC. http://www.epa.gov/osw/hazard/wastemin/priority.htm
  33. Usenko S, Landers DH, Appleby PG, Simonich SL (2007) Current and historical deposition of PBDEs, pesticides, PCBs, and PAHs to rocky mountain national park. Environ Sci Technol 41:7235-241 CrossRef
  34. Wang GD, Zhang Q, Ma P, Rowden J, Mielke HW, Gonzales C, Powell E (2008) Sources and distribution of polycyclic aromatic hydrocarbons in urban soils: case studies of Detroit and New Orleans. Soil Sediment Contam 17:547-63 CrossRef
  35. Wang Z, Yang P, Wang Y, Ma XD (2012) Urban fraction of polycyclic aromatic hydrocarbons from Dalian soils. Environ Chem Lett 10:183-87 CrossRef
  36. Wilcke W (2000) Polycyclic aromatic hydrocarbons (PAHs) in soil—a review. J Plant Nutr Soil Sci 163:229-48 CrossRef
  37. Wu SM, Yu WJ (2012) Liquid-liquid extraction of polycyclic aromatic hydrocarbons in four different edible oils from China. Food Chem 134:597-01 CrossRef
  38. Yunker MB, Macdonald RW, Vingarzan R, Mitchell RH, Goyette D, Sylvestre S (2002) PAHs in the Fraser river basin: a critical appraisal of PAH ratio as indicator of PAH source and composition. Org Geochem 33:489-15 CrossRef
  39. Zhu LZ, Chen YY, Zhou RB (2008) Distribution of polycyclic aromatic hydrocarbons in water, sediment and soil in drinking water resource of Zhejiang Province, China. J Hazard Mater 150:308-16 CrossRef
  
• 作者单位：Shoujun Yuan (1)
  Kebin Li (2)
  Tianhu Chen (3)
  Xiaolong Bi (4)
  Qiquan Wang (5)
  
  1. School of Civil and Hydraulic Engineering, Hefei University of Technology, Hefei, China
  2. School of Chemistry and Material Science, Northwest University, Xi’an, China
  3. School of Resources and Environmental Engineering, Hefei University of Technology, Hefei, China
  4. School of Energy and Power Engineering, Nanjing Institute of Technology, Nanjing, China
  5. Chemistry Department, Delaware State University, Dover, DE, 19901, USA
  
• ISSN：1866-6299

文摘

As a US east coast state with a major income from outdoor recreation and tourism, Delaware highly values its environmental quality and natural resources. However, no results on polycyclic aromatic hydrocarbons (PAHs) contamination in soil at natural recreational areas (NRAs) in the state have been reported. In this study soil samples from seven state parks, two city parks, two state forests, and two national wildlife refuges in Delaware were analyzed for the concentrations of 12 selected PAHs. Results indicated that the median concentration of total PAHs in urban, suburban, and rural NRAs was 1,159, 138, and 130?μg/kg, respectively. Based on the classification proposed by Maliszewska-Kordybach, soil PAH contamination level at almost all sampling sites in urban NRAs was classified as contaminated or heavily contaminated, while that at sampling sites in suburban and rural NRAs was classified as not or weakly contaminated. Principal component analysis showed that all these areas share the same independent variable, which may be composed of one or more contribution sources. Pyrogenic processes were inferred to be the major source of soil PAH contamination in Delaware NRAs. Individual PAH concentration at all sampling sites were observed below the limit of Canadian Quality Guidelines except for site F3, where the concentration of benzo[b]flouranthene, benzo[k]flouranthene, and benzo[a]pyrene was found to exceed the limit by 88.3, 125, and 281?%, respectively. Further investigation on PAH contamination and possible remediation in area F are recommended.