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Quantum criticality in NbFe2
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文摘
The C14 Laves phase NbFe2 is one of the few reported low temperature antiferromagnets among the transition metal compounds. It represents an interesting candidate for a study of antiferromagnetic quantum criticality in a strictly itinerant system. Because the nature of the ordered state in stoichiometric NbFe2 is still controversial—neutrons fail to pick up signatures of magnetic order, which are, however, detected using NMR—we have investigated the thermodynamic and transport properties of NbFe2 in a range of samples with near-stoichiometric composition. A large uniform susceptibility χ of the order of e52009c50a74e71401316510381a640"" title=""Click to view the MathML source"">1.8×10-2 (SI), which corresponds to a record Stoner enhancement factor of about 150, places all samples close to the threshold of ferromagnetism. Strongly field-dependent anomalies in the heat capacity and χ, however, point at spin-density-wave order below in stoichiometric NbFe2, indicating an intriguing interplay between ferromagnetism and antiferromagnetism. Slightly Nb-rich samples, which show no evidence of magnetic order, display distinct deviations from Fermi-liquid behaviour, consistent with close proximity to a magnetic quantum critical point.

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