Polydopamine (PD) played the multi-role as reducing agent, functionalizer, and favorable metal binder.
3D interconnected rGO/PD foam with controlled BET surface area was produced by controlling the degree of functionalized PD.
Optimum size, distribution, and loading amount of Pt in Pt-decorated rGO/PD could be systematically controlled.
High hydrogen uptake of rGO/PD_Pt (3.19 wt.%) was obtained at room temperature and 100 bar.
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