Recent Advances in Two-Dimensional Materials beyond Graphene

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• 作者：Ganesh R. Bhimanapati ; Zhong Lin ; Vincent Meunier ; Yeonwoong Jung ; Judy Cha ; Saptarshi Das ; Di Xiao ; Youngwoo Son ; Michael S. Strano ; Valentino R. Cooper ; Liangbo Liang ; Steven G. Louie ; Emilie Ringe ; Wu Zhou ; Steve S. Kim ; Rajesh R. Naik ; Bobby G. Sumpter ; Humberto Terrones ; Fengnian Xia ; Yeliang Wang ; Jun Zhu ; Deji Akinwande ; Nasim Alem ; Jon A. Schuller ; Raymond E. Schaak ; Mauricio Terrones ; Joshua A. Robinson
• 刊名：ACS Nano
• 出版年：2015
• 出版时间：December 22, 2015
• 年：2015
• 卷：9
• 期：12
• 页码：11509-11539
• 全文大小：2013K
• ISSN：1936-086X

文摘

The isolation of graphene in 2004 from graphite was a defining moment for the 鈥渂irth鈥?of a field: two-dimensional (2D) materials. In recent years, there has been a rapidly increasing number of papers focusing on non-graphene layered materials, including transition-metal dichalcogenides (TMDs), because of the new properties and applications that emerge upon 2D confinement. Here, we review significant recent advances and important new developments in 2D materials 鈥渂eyond graphene鈥? We provide insight into the theoretical modeling and understanding of the van der Waals (vdW) forces that hold together the 2D layers in bulk solids, as well as their excitonic properties and growth morphologies. Additionally, we highlight recent breakthroughs in TMD synthesis and characterization and discuss the newest families of 2D materials, including monoelement 2D materials (i.e., silicene, phosphorene, etc.) and transition metal carbide- and carbon nitride-based MXenes. We then discuss the doping and functionalization of 2D materials beyond graphene that enable device applications, followed by advances in electronic, optoelectronic, and magnetic devices and theory. Finally, we provide perspectives on the future of 2D materials beyond graphene.