Electrocatalytic degradation of bisphenol a in aqueous solution using β-PbO2/Ti as anode

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• 作者：Chengzhu Zhu ; Caiju Hu ; Jun Lu ; Xiaohui Wang…
• 关键词：β ; PbO2 anode ; electrocatalytic degradation ; bisphenol A ; OH radicals
• 刊名：Russian Journal of Electrochemistry
• 出版年：2015
• 出版时间：April 2015
• 年：2015
• 卷：51
• 期：4
• 页码：353-361
• 全文大小：438 KB
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• 作者单位：Chengzhu Zhu (1)
  Caiju Hu (1)
  Jun Lu (2)
  Xiaohui Wang (1)
  Li Huang (3)
  Tianhu Chen (1)
  
  1. School of Resources and Environmental Engineering, Hefei University of Technology, Hefei, 230009, P.R. China
  2. Center of Analysis and Measurement, Hefei University of Technology, Hefei, 230009, P.R. China
  3. Wadsworth Center, New York State Department of Health, Albany, NY, 12201-0509, USA
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Electrochemistry
  Physical Chemistry
  Russian Library of Science
  
• 出版者：MAIK Nauka/Interperiodica distributed exclusively by Springer Science+Business Media LLC.
• ISSN：1608-3342

文摘

In this paper, a novel Ti-base β-PbO₂ electrode was successfully prepared by using electrodeposition. The prepared electrode was characterized by scanning electron microscopy (SEM), X-ray diffraction (XRD) and anode polarization curves. The electrocatalytic degradation efficiency of bisphenol A by using the novel Ti-base β-PbO₂ as anode were examined as a function of supporting electrolyte types and concentrations, electrolysis time, initial BPA concentration, initial pH and current efficiency. The results showed that the removal efficiency of COD_Cr could reach up to 90.6% after 1.5-h electrolysis at initial bisphenol A concentration of 20 mg L?, applied voltage of 20 V, electrode spacing of 7 cm, initial pH of 5, and NaCl concentration of 0.020 mol L?. The electrocatalytic degradation of bisphenol A was induced by hydroxyl radical and other oxidative species attacking parent molecules. The degradation products mainly consisted of small straight chain compounds, CO₂ and H₂O.