Electrochemical Sensor based on Imprinted Sol-Gel Polymer on Au NPs-MWCNTs-CS Modified Electrode for the Determination of Acrylamide

详细信息    查看全文

• 作者：Xia Liu ; Lu-Gang Mao ; Yuan-Liang Wang ; Xing-Bo Shi ; Yan Liu…
• 关键词：Electrochemical sensor ; Acrylamide ; Gold nanoparticles ; Chitosan ; Multiwalled carbon nanotubes ; Sol ; gel molecularly imprinted
• 刊名：Food Analytical Methods
• 出版年：2016
• 出版时间：January 2016
• 年：2016
• 卷：9
• 期：1
• 页码：114-121
• 全文大小：946 KB
• 参考文献：Backe WJ, Yingling V, Johnson T (2014) The determination of acrylamide in environmental and drinking waters by large-volume injection-hydrophilic-interaction liquid chromatography and tandem mass spectrometry. J Chromatogr A 1334:72–78CrossRef
  Bagdonaite K, Derler K, Murkovic M, Agric J (2008) Determination of Acrylamide during Roasting of Coffee. Food Chem 56:6081–6086CrossRef
  Blanch GP, Morales FJ, Moreno FP, Castillo MLR (2013) A new approach based on off-line coupling of high-performance liquid chromatography with gas chromatography-mass spectrometry to determine acrylamide in coffee brew. J Sep Sci 36:320–324CrossRef
  David AG, Dwight SS, Weston LD, Matthew DM, Pinal CP, Chad AM (2010) Gold nanoparticles for biology and medicine. Angew Chem Int Ed 49:3280–3294CrossRef
  Gong X (2013) Controlling surface properties of polyelectrolyte multilayers by assembly pH. Phys Chem Chem Phys 15:10459CrossRef
  Gong X (2014) Facile formation of nanoparticle patterns by water induced flow of a polymer thin film. Res Adv 4:54494
  Grabar KC, Smith PC, Musick MD, Davis JA, Walter DG, Jackson MA, Guthrie AP, Natan MJ (1996) Kinetic Control of Interparticle Spacing in Au Colloid-Based Surfaces: Rational Nanometer-Scale Architecture. J Am Chem Soc 118:1148–1153CrossRef
  Hu YF, Zhang ZH, Zhang HB, Luo LJ, Yao SZ (2011) Electrochemical determination of L-phenylalanine at polyniline modified carbon electrode based on β-cyclodextrin incorporated carbon nanotube composite material and imprinted sol-gel film. Talanta 84:305–313CrossRef
  Huang JD, Zhang XM, Lin Q, He XR, Xing XR, Huai HX, Lian WJ, Zhu H (2011) Electrochemical sensor based on imprinted sol-gel and nanomaterials for sensitive determination of bisphenol A. Food Control 22:786–791CrossRef
  International Food Safety Authorities Network (INFOSAN) Information Note No. 2. Acrylamide in food is a potential health hazard. Geneva, Switzerland, 1st March, 2005, http://​www.​fsai.​ie/​industry/​hottopics/​EN.​note2.​2005.​acrylamide.​Pdf
  Marx S, Zaltsman A, Turyan I, Mandler D (2004) Preparation sensor based on molecularly imprinted sol-gel films. Anal Chem 76:120–126CrossRef
  Mottram DS, Wedzicha BL, Dodson AT (2002) Food chemistry: acrylamide is formed in the Maillard reaction. Nature 419:448–449CrossRef
  Prasad BB, Madhuri R, Tiwari MP, Sharma PS (2010) Electrochemical sensor for folic acid based on a hyperbranched molecularly imprinted polymer-immobilized sol-gel-modified pencil graphite electrode. Sens Actuators B 146:321–330CrossRef
  Qin X, Wang HC, Wang XS, Miao ZY, Chen LL, Zhao W (2010) Amperometric biosensors based on gold nanoparticles-decorated multiwalled carbon nanotubes-poly biocomposite for the determination of choline. Sens Actuators B 147:593–598CrossRef
  Rezaei B, Boroujeni MK, Ensafi AA (2014) Caffeine electrochemical sensor using imprinted film as recognition element based on polypyrrole sol-gel and gold nanoparticles hybrod nanocomposite modified pencil graphite electrode. Biosens Bioelectron 60:77–83CrossRef
  Riskin M, Tel-Vered R, Bourenko T, Granot E, Willner I (2008) Imprinting of molecular recognition sites through electropolymerization of functionalized Au nanoparticles: development of an electrochemical TNT Sensor Based on π-Donor − Acceptor Interactions. J Am Chem Soc 130:9726–9733CrossRef
  Saha K, Agasti S, Kim C, Li XN, Rotello VM (2012) Gold nanoparticles in chemical and biological sensing. Chem Rev 112:2739–2779CrossRef
  Soares C, Cunha C, Fernandes J (2006) Determination of acrylamide in coffee and coffee products by GC-MS using an improved SPE clean-up. Food Addit Contam 23:1276–1282CrossRef
  Stadler RH, Blank I, Varga N, Robert F (2002) Food chemistry: acrylamide from Maillard reaction products. Nature 419:449–450CrossRef
  Suginta W, Khunkaewla P, Schulte A (2013) Electrochemical biosensor applications of polysaccharides chitin and chitosan. Chem Rev 113:5458–5479CrossRef
  Wang ZH, Li JS, Liu XL, Yang JM, Lu XQ (2013) Preparation of an amperometric sensor for norfloxacin based on molecularly imprinted grafting photopolymerization. Anal Bioanal Chem 405:2525–2533CrossRef
  Wang X, Piro B, Reisberg S, Anquetin G, Rocquigny HD, Jiang P, Wang Q, Wu W, Pham MC, Dong CZ (2014a) Direct, reagentless electrochemical detection of the BIR3 domain of X-linked inhibitor of apoptosis protein using a peptide-based conducting polymer sensor. Biosens Bioelectron 61:57–62CrossRef
  Wang QY, Ji J, Jiang DL, Wang Y, Zhang YZ, Sun XL (2014b) An electrochemical sensor based on molecularly imprinted membranes on a P-ATP–AuNP modified electrode for the determination of acrylamide. Anal Methods 6:6452CrossRef
  WTO (1993) Guidelines for drinking water quality [R]. WHO: World Health Organization
  Xu HF, Dai H, Chen GN (2010) Direct electrochemistry and electrocatalysis of hemoglobin protein entrapped in grahene and chirosan composite film. Talanta 81:334–338CrossRef
  Xu W, Liu P, Guo GH, Dong C, Zhang XH, Wang SF (2013) Electrochemical sensor based on a carbon nanotube-modified imprinted sol-gel for selective and sensitive determination of β2-agonists. Microchim Acta 180:1005–1011CrossRef
  Xu GL, Zhang HL, Zhong M, Zhang TT, Lu XJ, Kan XW (2014) Imprinted sol-gel electrochemical sensor for melamine direct recognition and detection. J Electroanal Chem 713:112–118CrossRef
  Yang YK, Fang GZ, Liu GY, Pan MF, Wang XM, Kong LJ, He XL, Wang S (2013) Electrochemical sensor based on molecularly imprinted polymer film via sol-gel technology and multi-walled carbon nanotubes-chitosan functional layer for sensitive determination of quinoxaline-2-carboxylic acid. Biosens Bioelectron 47:475–481CrossRef
  Yuan Y, Zhao GH, Hu XX, Wu JH, Liu J, Chen F (2008) High correlation of methylglyoxal with acrylamide formation in glucose/asparagine Maillard reaction model. Eur Food Res Technol 226:1301–1307CrossRef
  Zhang ZH, Hu YF, Zhang HB, Luo LJ, Yao SZ (2010) Layer-by-layer assembly sensitive electrochemical sensor for selectively probing L-histidine based on molecular imprinting sol-gel at functionalized indium tin oxide electrode. Biosens Bioelectron 26:696–702CrossRef
  Zhang J, Niu YH, Li SJ, Luo RQ, Wang CY (2014) A molecularly imprinted electrochemical sensor based on sol-gel techenogology and multiwalled carbon nanotubes-Nafion functional layer for determination of 2-nonylphenol in environmental samples. Sens Actuators B 193:844–850CrossRef
  Zhu AH, Xu GL, Li L, Yang LL, Zhou H, Kan XW (2013) Sol-gel imprinted polymers based electrochemical sensor for paracetamol recognition and detection. Anal Lett 46:7
  Zhu Y, Zeng GM, Zhang Y, Tang L, Chen J, Cheng M (2014) Highly sensitive electrochemical sensor using a MWCNTs/Au NPs-modified electrode for lead(II) detection based on Pb2+-induced G-rich DNA conformation. Analyst 139:5014–5020CrossRef
  
• 作者单位：Xia Liu (1)
  Lu-Gang Mao (1)
  Yuan-Liang Wang (1)
  Xing-Bo Shi (1)
  Yan Liu (1)
  Yang Yang (1)
  Zao He (1)
  
  1. College of Food Science and Technology, Hunan Agricultural University, Hunan Province Key Laboratory of Food Science and Biotechnology, Changsha, 410128, People’s Republic of China
  
• 刊物类别：Chemistry and Materials Science
• 刊物主题：Chemistry
  Food Science
  Chemistry
  Microbiology
  Analytical Chemistry
  
• 出版者：Springer New York
• ISSN：1936-976X

文摘

A sensitive molecularly imprinted electrochemical sensor was successfully constructed for the detection of acrylamide (AM). It is based on a glassy carbon electrode modified with a composites prepared from gold nanoparticles, multiwalled carbon nanotubes, and chitosan along with a sol-gel-based molecularly imprinted polymer (MIP) film. The latter was prepared using AM as the template molecule, 3-aminopropyltrimethoxysilane as the functional monomer, and tetraethoxysilane as the cross-linker. The MIP sensor showed a linear current response to the target AM concentration in the range from 0.05 to 5 μg mL−1 at a working voltage of 0–0.4 V with a lower detection limit of 0.028 μg mL−1 (S/N = 3). It was successfully applied to the detection of AM in potato chips. HPLC analysis was also conducted to detect AM in the same samples to demonstrate the applicability of the electrochemical MIP sensor. Keywords Electrochemical sensor Acrylamide Gold nanoparticles Chitosan Multiwalled carbon nanotubes Sol-gel molecularly imprinted