长江>望虞河入贡湖处>贡湖内",其与调水过程中颗粒物沉降作用及自然来源磷的输入有关。贡湖内悬浮颗粒物中弱吸附态磷、可提取态有机磷、铁结合态磷含量低于长江、望虞河段,然而其3者含量之和占颗粒态总磷的质量分数高于长江段,这跟贡湖内水体中藻类生长情况相对于长江比较旺盛有关。" />
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引江济太调水河段悬浮颗粒物中磷的形态与分布研究
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摘要
2013年8月引江济太调水期间,采集调水河段长江-望虞河-贡湖表层水样,经0.45μm滤膜过滤处理得到悬浮颗粒物样品,开展悬浮颗粒物中磷形态(弱吸附态磷、可提取态有机磷、铁结合态磷、自生磷灰石磷、碎屑磷和非活性磷)的含量及空间分布特征研究。结果表明,长江-望虞河-贡湖段水体悬浮颗粒物中颗粒态总磷的含量范围为284.85μg/g-1814.12μg/g,主要以碎屑磷和非活性磷形态赋存,其含量之和平均占颗粒态总磷含量的56.95%。颗粒态总磷、自生磷灰石磷、碎屑磷和非活性磷含量的空间分布特征为"望虞河起始段>长江>望虞河入贡湖处>贡湖内",其与调水过程中颗粒物沉降作用及自然来源磷的输入有关。贡湖内悬浮颗粒物中弱吸附态磷、可提取态有机磷、铁结合态磷含量低于长江、望虞河段,然而其3者含量之和占颗粒态总磷的质量分数高于长江段,这跟贡湖内水体中藻类生长情况相对于长江比较旺盛有关。
surface water were collected from the Yangtze River, the Wangyu River and the Gong Lake during diversion from the Yangtze River to the Tai Lake in August 2013, and were filtered through 0.45μm filter membranes to get samples of suspended particulate matters. The phosphorus in the suspended particulate matters were divided into six forms, which were exchangeable phosphorus(Ex-P), exchangeable organic phosphorus(Ex-Org-P), iron-bound phosphorus(Fe-P), authigenic phosphorus(Ca-P), detrital phosphorus(HCl-P), and refractory phosphorus(Res-P), and their concentration distributions were analyzed. The results indicated that the concentration range of the total phosphorus in the study area was 284.85μg/g~1814.12μg/g.The HCl-P and Res-P were the main forms and their sum concentration took up 56.95% of the total phosphorus of particulate matters. The space distribution characteristics of the total phosphorus of particulate matters, the Ca-P, the HCl-P, the Res-P were influenced by settlement actions of particulate matters during diversion process and inputs of natural phosphorus sources, and their concentrations in the study area showed the following decreasing order: the primary section of the Wangyu River > the Yangtze River > the Wangyu River falling into the Gong Lake > the Gong Lake. The concentrations of Ex-P, Ex-Org-P and Fe-P in the Gong Lake were lower than concentrations in the Yangtze River and the Wangyu River. However, the sum percentage of the Ex-P, Ex-Org-P and Fe-P taking up the total phosphorus of particulate matters in the Gong Lake, was higher than that of percentage in the Yangtze River. This was related to more excessive phytoplankton growth in the Gong Lake than the Yangtze River.
引文
[1]Michel Meybeck.Carbon,nitrogen and phosphorus transport by world rivers[J].American Journal of Science,1982,282:401-450.
    [2]Jukka Horppila,Leena Nurminen.The effect of an emergent macrophyte(Typha angustifolia)on sediment resuspension in a shallow north temperate lake[J].Freshwater Biology,2001,46(11):1447-1455.
    [3]赵颖,王国秀,章北平.典型城内过富营养化湖泊沉积物和间隙水中各形态磷的相关性研究[J].长江流域资源与环境,2006,15(4):490-494.
    [4]K Pettersso.Phosphorus characteristics of setting and suspended particles in Lake Erken[J].Sci Total Environ,2001,266(1-3):79-86.
    [5]Martin Sondergaard,Jens Peder Jensen,Erik Jeppesen.Role of sediment and internal loading of phosphorus in shallow lakes[J].Hydrobiologia,506-509(1-3):135-145.
    [6]刘春生,吴浩云.引江济太调水试验的理论和实践探索[J].水利水电技术,2003,34(1):4-8.
    [7]燕姝雯,余晖,张璐璐,徐军,王振平.2009年环太湖入出湖河流水量及污染负荷通量[J].湖泊科学,2011,23(6):855-862.
    [8]Kathleen C Ruttenberg.Development of a sequential extraction method for different forms of phosphorus in marine sediments[J].Limnology and Oceanography,1992,37(7):1460-1482.
    [9]刘鹏霞.三峡水库蓄水至135米后库区和长江干流各形态磷的分布特征研究[J].青岛:中国海洋大学,2007:1-22.
    [10]何会军.河流与河口颗粒物中磷的生物地球化学特征研究[D].青岛:中国海洋大学,2009:35-44.
    [11]T J Logan.Mechanism for release of sediment-bound phosphate to water and the effects of agricultural land and management on fluvial transport of particulate and dissolved phosphate[J].Hydrobiologia,1982,91-92(1):519-530.
    [12]孟佳,姚庆祯,陈洪涛,于志刚.北黄海表层沉积物中颗粒态磷的形态分布[J].环境科学,2012,33(10):3361-3367.
    [13]李悦,乌大年,薛永先.沉积物中不同形态磷提取方法的改进及其环境地球化学意义[J].海洋环境科学,1998,17(1):15-20.
    [14]V.Ruban,J.F.Lopez-Sanchez,P.Pardo,G.Rauret,H.Muntau,Ph.Quevauviller.Selection and evaluation of sequential extraction procedures for the determination of phosphorus forms in lake sediment[J].Journal of Environmental Monitoring,1999,1(1):51-56.
    [15]许春雪,袁建,王亚平,王苏明,代阿芳.沉积物中磷的赋存形态及磷形态顺序提取分析方法[J].岩矿测试,2011,30(6):785-794.
    [16]魏俊峰,陈洪涛,刘鹏霞,李荣华,于志刚.长江悬浮颗粒物中磷的赋存形态[J].水科学进展,2010,21(1):107-112.
    [17]魏俊峰,陈洪涛,刘月良,单凯,姚庆祯,何会军,于志刚.2008年调水调沙期间黄河下游悬浮颗粒物中磷的赋存形态[J].环境科学,2011,32(2):368-374.
    [18]李珊珊,郭沛涌,童敏,李林蔚,王进铭.厦门石兜-坂头水库悬浮颗粒物中磷形态的分布特征及其与叶绿素a的相关性[J].生态学杂志,2010,29(10):1979-1984.
    [19]杨逸萍,胡明辉.河口悬浮物种磷的化学形态分布与转化[J].台湾海峡,1995,14(4):313-319.
    [20]高永霞,蔡琳琳,赵林林,朱广伟.丰水期环太湖河流与湖区水质比较研究[J].环境科学,2011,32(10):2840-2848.

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